A reference for the density of singular K3 surfaces in the period domain (see Will Sawin's answer) is
Piatetski-Shapiro, Ilya I.; Shafarevich, I. R., Arithmetic of K3 surfaces, Trudy Mezhdunarod. Konf. Teor. Chisel, Moskva 1971, Tr. Mat. Inst. Steklova 132, 44-54 (1973) ZBL0293.14010.
In particular, this is a screenshot of page 54: