The answer by Jules Lamers considers $k=1$.
In the comments to that answer, people have mentioned that the case $k=0$ has been solved. Namely, for a given partition $\lambda$ let Del($\lambda$) be the set of boxes in its diagram that may be deleted and the result is still a diagram. Then
$$ L_0(s_\lambda)=\sum_{\square \in {\rm Del}(\lambda)} [c(\square)+N]s_{\lambda-\square},$$
where $N$ is the number of variables, $ c(\square)$ is the content of a box and $\lambda-\square$ is the diagram obtained from $\lambda$ upon deletion of that box.
I have done some experimentation, and I would like to propose a conjecture for the action of $L_2$ on a Schur polynomial.
Let Ins($\lambda$) be the set of boxes that may be inserted in its diagram and the result is still a diagram. Then I believe that
$$ L_2(s_\lambda)=\sum_{\square \in {\rm Ins}(\lambda)} c(\square)s_{\lambda+\square}.$$
For example, in the diagram for $(2,1)$ three boxes can be inserted, leading to either $(3,1)$, $(2,2)$ or $(2,1,1)$. In the first case the content of the inserted box is $2$, in the second case it is $0$ and in the third case it is $-2$. So $L_2(s_{(2,1)})=2s_{(3,1)}+0s_{(2,2)}-2s_{(2,1,1)}.$
I would be grateful if someone could prove this. Such a simple result cannot be too hard.