Space-level homotopy induces (co)chain homotopy, but I've never heard of the converse. I am not sure if it is simply not true?
However, for good enough spaces (finite type nilpotent), Mandell proved that weak homotopy types are determined by cochain complexes as an $E_\infty$-algebras up to quasi-isomorphism. Does this suggest that there are (co)chain homotopies in the sense of $E_\infty$, such that all of them backward induce homotopies between maps between spaces?