I will formulate this question in the language of Jacobi operators and spectral measures although it could be entirely rewritten in terms of orthogonal polynomials and measures of orthogonality.
Objects of interest: Let $J$ be a semi-infinite Jacobi matrix of the form $$J=\begin{pmatrix} b_{1} & a_{1}\\ a_{1} & b_{2} & a_{2}\\ & a_{2} & b_{3} & a_{3}\\ & & \ddots & \ddots & \ddots \end{pmatrix},$$ where $b_{n}\in\mathbb{R}$ and $a_{n}>0$. Let $\mathcal{M}$ denotes the set of Jacobi matrices $J$ such that $b_{n}\to 0$ and $a_{n}\to 1$ as $n\to\infty$ (the so-called Szegö class in OG polynomials terminology).
Let $J_{0}$ be the Jacobi matrix with $b_{n}=0$ and $a_{n}=1$ for all $n\in\mathbb{N}$. It is well-known that the spectrum of $J_{0}$ is $$\sigma(J_{0})=[-2,2].$$ A Jacobi matrix $J\in\mathcal{M}$ iff $J-J_{0}$ is compact.
For any self-adjoint operator $J$ (assume $J$ is bounded), there exists unique measure $\mu$ (the spectral measure) determined by the equality $$\int_{\mathbb{R}}\frac{d\mu(x)}{x-z}=\langle e_{1},(J-z)e_{1}\rangle, \quad \forall z\in\mathbb{C}\setminus\mathbb{R},$$ where $e_{1}$ is the first vector of the standard basis of $\ell^{2}(\mathbb{N})$. It holds that $\mbox{supp}\mu=\sigma(J)$.
Question: Assume $\mu$ to be a probability measure with $\mbox{supp}\mu=[-2,2]$. Then there exists a unique Jacobi operator $J$ whose spectral measure coincides with $\mu$. I am interested in what additional conditions (to $\mbox{supp}\mu=[-2,2]$) is to be imposed on the measure $\mu$ to guarantee that $J\in\mathcal{M}$. The condition (if any) should be weaker than the Szegö condition which gives us more, see below.
What is known: There is an answer to this kind of question known for a long time but it implies even more than just $J\in\mathcal{M}$. Namely, if $\mbox{supp}\mu=[-2,2]$ and the density $\rho$ of the the Lebesgue absolutely continuous component of $\mu$ satisfies the so-caled Szegö condition: $$\int_{-2}^{2}\frac{\log\rho(x)}{\sqrt{4-x^{2}}}dx>-\infty,$$ then $$\sum_{n=1}^{\infty}b_{n}^{2}<\infty \quad \mbox{ and } \quad \sum_{n=1}^{\infty}(a_{n}-1)^{2}<\infty.$$ In particular, $J\in\mathcal{M}$. Proof and references for these claims (and much more) can be found here.