It is an elementary fact that a map $f:X \to Y$ between spaces induces a chain complex morphism $f_* : C_*(X) \to C_*(Y) $. This allows one to transfer 1-category theoretic arguments from spaces to associated chain complexes.
When dealing with $\infty$ stuff, sometimes a bit more is needed. Let $\textrm{Sing}(\textrm{Top})$ be the simplicially enriched category of topological spaces with
$$Map_{\textrm{Top}}(X, Y) _n = Hom_{\textrm{Top}}(X \times \Delta^n, Y) $$
And let $\textrm{Ch}(\mathbb{Z}) $ be the simplicially enriched category of chain complexes with
$$Map_{\textrm{Ch}(\mathbb{Z})}(C, D) = Hom_{\textrm{Ch}(\mathbb{Z})}(C \otimes \mathbb{Z}[\Delta^n], D) $$
where $\mathbb{Z}[\Delta^n]$ is the simplicially chain complex of $\Delta^n$: it has in degree $k$ the span of its $k$ dimensional faces.
Is it true that $C_*$ is a simplicial functor from $\textrm{Top}$ to $\textrm{Ch}(\mathbb{Z})$?
I thought this was almost tautological, but there are some Alexander Whitney and Eilenberg-Zilber maps involved that are not straightforward. A reference would be highly appreciated. I couldn't find this in HTT, but maybe it's me. As a remark, let me say the above functor factors explicitly through simplicial abelian complexes, so the crucial point is probably in the Dold-Kan part.
In case this is not true:
Informally, how one can transfer $\infty$ arguments from spaces to chain complexes? For example, is there a quasi-isomorphic functor to $C_*$ that becomes simplicial?