The Curlcurl of a vector field $X=P\partial_x+Q\partial_y+R\partial_z$ is equal to $$Curl X= (R_y-Q_z)\partial_x +(P_z-R_x)\partial_y+ (Q_x-P_y)\partial_z$$
$$
\mathrm{Curl}(X)= (R_y-Q_z)\,\partial_x +(P_z-R_x)\,\partial_y+ (Q_x-P_y)\,\partial_z
$$
For the moment we replace $\partial_x,\partial_y,\partial_z$ with $dy\wedge dz, dx\wedge dz, dx\wedge dy$$dy\wedge dz,\ dx\wedge dz$ and $dx\wedge dy$ respectively. (In fact we apply the Hodge star operator to the dual of the base basis $\partial_x,\partial_y,\partial_z$).
So actually the component of $Curl X$$\mathrm{Curl}(X)$ is identical to the compenents components of the $2$ form $$\alpha=(R_y-Q_z)dy\wedge dz +(P_z-R_x)dx\wedge dz +(Q_x-P_y)dx\wedge dy$$ $$ \alpha=(R_y-Q_z)\,dy\wedge dz +(P_z-R_x)\,dx\wedge dz +(Q_x-P_y)\,dx\wedge dy $$
On the other hand the vector field $X$, being a section of the tangent bundle $T\mathbb{R}^3$, can be considered as a map $$X:\mathbb{R}^3 \to \mathbb{R}^3\times \mathbb{R}^3\\X(x,y,z)=(x,y,z, P(x,y,z),Q(x,y,z),R(x,y,z))$$.
\begin{align}
X\colon \mathbb{R}^3& \to \mathbb{R}^3\times \mathbb{R}^3\\
(x,y,z)&\mapsto (x,y,z, P(x,y,z),Q(x,y,z),R(x,y,z)).
\end{align}
Note that the following equality holdholds:
$$\alpha =X^* \omega$$ where
$$
\alpha =X^* \omega,
$$
where $\omega$ is the natural symplectic structure of $\mathbb{R}^3 \times \mathbb{R}^3$ with $\omega= dx\wedge dp +dy\wedge dq+dz \wedge dr$.
The situation described above is a motivation to consider the following generalization of the concept of the Curl curl of a vector field on an arbitraryarbitrary Riemannian manifold.
A generalized Curlcurl: Let $(M,g)$ be a Riemannian manifold. The metric $g$ gives an isomorphism (hence diffeomorphism) between $TM$ and $T^* M$. So the standard intrinsic symplectic structure of the cotangant cotangent bundle is carried to a symplectic structure $\omega$ on $TM$. Now assume that $X:M \to TM$ is a vector field. We define the Curle curl of $X$ as a $2$-form with the following formula $$Curl X=X^* \omega$$: $$ \mathrm{Curl}(X):=X^* \omega. $$
This is was already mentioned at thisthe MO question.
A generalization of Gradient vector fields and Curl of vector fields.