Two easy observations: (1) If $C$ has (box counting) dimension $<1/2$, then the chord set doesn't even have positive area. This is mentioned in the linked question, but just to make the trivial argument explicit, here it is: cover $C$ by $N\gg 1$ intervals of length $\le \ell$ each. For a fixed pair of intervals, the corresponding chords have area $\lesssim \ell$, so the total area is $\lesssim N^2\ell\to 0$ (since $N\lesssim\ell^{-1/2+\epsilon}$ under our current assumptions).
(2) There are Cantor sets for which the chord set is convex. This follows from the observation that if $n$ open intervals have already been deleted and the current chord set is convex, then we can delete one more (small) interval at the center of the largest remaining arc in such a way that the chord set remains convex.
To see this, just deletelet's survey the center itself and lookdamage done by deleting a small interval at the (triangular) regionscenter of chords that have now disappearedone of our arcs. We need alternativeFix one of the other arcs and consider all the chords to still coverstarting at that arc that are no longer available because they end in the same pointsdeleted interval. We're definitely good close toWhen the distance from the deleted pointinterval gets larger than a certain small critical distance $d$, thanks tothese points are still all covered by using nearby endpoints from the remaining parts of theour arc from which weinstead of the deleted ones. At some distance from our pointMoreover, $d\to 0$ as we have some positive amount of space to maneuver becauseshrink the partner point isdeleted interval. We do slice off the region bounded by the deleted arc and its secant. Other than this, points that are close are still covered by going from one half of finitely many intervalswhat remains of positive minimum lengththe original arc to the other. So we see that we may delete a whole interval, as long as thisWe need to take our interval staysso small that all $d$'s (corresponding to the finitely many other intervals) are smaller than the minimum optional wiggling length that is obtained in this waydistance.